OoT
I liked the forest temple, and the spirit temple was alright,
but I LOVED the shadow temple. So atmospheric! So mysterious! So enthralling!
The visuals were tight and cool. I also like how everything was invisible/illusory.
My favorite was the Water Temple from Ocarina of Time. It was just a great temple with the design and the illusion of being underwater seemed to blend seemlessly to me.
The forest temple had a great atmosphere- although the newer Zeldas have greater looking temples, that one was the first to really blow me away (since the first three in OOT were cool looking but too quick and easy to leave a lasting impression)